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- Charles Lee Smith (1887–1964), American atheist activist
- Charlie Smith (centenarian) (1842 or 1874–1979), claimed to be the oldest person in the United States
- Charles Pressley Smith (1862–1935), Anglican priest
- Charles John Smith (1803–1838), English engraver
- Charles Rattray Smith (1859–1941), schoolteacher in Britain and New South Wales, Australia
- Charles Smith (developer) (1901–1995), real estate developer and philanthropist in the Washington DC area
- Charles Edward Smith (1835–?), American author and Baptist ecclesiologist and apologist
- Charles R. Smith, head of the Menasha Wooden Ware Co., who named Ladysmith, Wisconsin after his wife
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