- Antony Baekeland, grandson of Leo Baekeland, after his trial for stabbing his mother to death.
- Ian Ball, who attempted to kidnap Princess Anne in 1974
- William Rutherford Benn, father of Margaret Rutherford
- Ian Brady
- Charles Bronson
- Sharon Carr, who stabbed her first victim Katie Rackliff when she was just 12
- David Copeland
- Richard Dadd
- Gregory Davis
- Ibrahim Eidarous, alleged member of al-Jihad
- Kenneth Erskine
- June and Jennifer Gibbons
- Daniel Gonzalez
- James Kelly, convicted of killing his wife, suspected of being Jack the Ripper, his memoirs place his whereabouts around other unsolved murders in the UK and the United States.
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- Ronald Kray
- Thomas John Ley
- Robert Maudsley
- Roderick McLean
- Dr. William Chester Minor, known as The Surgeon of Crowthorne
- Daniel M'Naghten
- Robert Napper
- Edward Oxford
- Nicky Reilly
- John Straffen
- Peter Sutcliffe, known as the Yorkshire Ripper
- Roy Shaw
- Ronald True
- Graham Young, released by hospital as "fully recovered", and who later poisoned dozens of people, two fatally. Jailed aged 14 (youngest prisoner detained there since 1885).
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