Higher-order Frequency Mixing
The above holds for processes. It can be extended for processes where is nonzero, something that is generally true in any medium without any symmetry restrictions. Third-harmonic generation is a process, although in laser applications, it is usually implemented as a two-stage process: first the fundamental laser frequency is doubled and then the doubled and the fundamental frequencies are added in a sum-frequency process. The Kerr effect can be described as a as well.
At high intensities the Taylor series, which led the domination of the lower orders, does not converge anymore and instead a time based model is used. When a noble gas atom is hit by an intense laser pulse, which has an electric field strength comparable to the Coulomb field of the atom, the outermost electron may be ionized from the atom. Once freed, the electron can be accelerated by the electric field of the light, first moving away from the ion, then back toward it as the field changes direction. The electron may then recombine with the ion, releasing its energy in the form of a photon. The light is emitted at every peak of the laser light field which is intense enough, producing a series of attosecond light flashes. The photon energies generated by this process can extend past the 800th harmonic order up to 1300 eV. This is called high-order harmonic generation. The laser must be linearly polarized, so that the electron returns to the vicinity of the parent ion. High-order harmonic generation has been observed in noble gas jets, cells, and gas-filled capillary waveguides.
Read more about this topic: Nonlinear Optics
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