Cast
- Sean Connery as James Bond: Secret Intelligence Service Agent 007.
- Daniela Bianchi as Tatiana Romanova (voiced by Barbara Jefford): Soviet Embassy clerk and Bond's love interest. Fleming based Romanova on Christine Granville.
- Pedro Armendáriz as Ali Kerim Bey: British Intelligence Station Chief in Istanbul.
- Lotte Lenya as Rosa Klebb: Main villain and ex-SMERSH Colonel, now Chief Operations Officer for SPECTRE.
- Robert Shaw as Red Grant: Cunning SPECTRE assassin and one of the principal Bond enemies.
- Bernard Lee as M: Chief of British Intelligence.
- Walter Gotell as Morzeny: SPECTRE thug who trains personnel on SPECTRE Island.
- Vladek Sheybal as Kronsteen: Chess grandmaster, and Chief Planning Officer for SPECTRE.
- "?" (anonymous credit for Anthony Dawson (body) and Eric Pohlmann (voice)) as "Number 1" (Ernst Stavro Blofeld): Chief of SPECTRE and Bond's nemesis.
- Lois Maxwell as Miss Moneypenny: M's secretary.
- Desmond Llewelyn as Major Boothroyd: Head of 'Q' Section (British Intelligence gadgetry department).
- Eunice Gayson as Sylvia Trench: Bond's semi-regular girlfriend.
- Francis de Wolff as Vavra: Chief of a Gypsy tribe used for dirty work by Kerim Bey
- George Pastell as the Orient Express train conductor.
- Fred Haggerty as Krilencu: A Bulgarian assassin who works as a killer for the Soviets in The Balkans.
- Aliza Gur and Martine Beswick as Vida and Zora, respectively: Two jealous Gypsy girls who are disputing the same man.
- Nadja Regin as Kerim Bey's lonely girlfriend.
Read more about this topic: From Russia With Love (film)
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