Free-electron Laser - X-ray Uses

X-ray Uses

The lack of suitable mirrors in the extreme ultraviolet and x-ray regimes prevents the operation of a FEL oscillator; consequently, there must be suitable amplification over a single pass of the electron beam through the undulator to make the FEL worthwhile. X-ray free electron lasers use long undulators. The underlying principle of the intense pulses from the X-ray laser lies in the principle of self-amplified stimulated emission (SASE), which leads to the microbunching of the electrons. Initially all electrons are distributed evenly and they emit incoherent spontaneous radiation only. Through the interaction of this radiation and the electrons' oscillations, they drift into microbunches separated by a distance equal to one radiation wavelength. Through this interaction, all electrons begin emitting coherent radiation in phase. In other words, all emitted radiation can reinforce itself perfectly whereby wave crests and wave troughs are always superimposed on one another in the best possible way. This results in an exponential increase of emitted radiation power, leading to high beam intensities and laser-like properties. Examples of facilities operating on the SASE FEL principle include the Free electron LASer (FLASH) in Hamburg, the Linac Coherent Light Source (LCLS) at the SLAC National Accelerator Laboratory, the European x-ray free electron laser (XFEL) in Hamburg, the SPring-8 Compact SASE Source (SCSS), the SwissFEL at the Paul Scherrer Institute (Switzerland) and, as of 2011, the SACLA at the RIKEN Harima Institute in Japan.

One problem with SASE FELs is the lack of temporal coherence due to a noisy startup process. To avoid this, one can "seed" an FEL with a laser tuned to the resonance of the FEL. Such a temporally coherent seed can be produced by more conventional means, such as by high-harmonic generation (HHG) using an optical laser pulse. This results in coherent amplification of the input signal; in effect, the output laser quality is characterized by the seed. While HHG seeds are available at wavelengths down to the extreme ultraviolet, seeding is not feasible at x-ray wavelengths due to the lack of conventional x-ray lasers. In late 2010, in Italy, the seeded-FEL source FERMI@Elettra has started commissioning, at the Sincrotrone Trieste Laboratory. FERMI@Elettra is a single-pass FEL user-facility covering the wavelength range from 100 nm (12 eV) to 10 nm (124 eV), located next to the third-generation synchrotron radiation facility ELETTRA in Trieste, Italy. The advent of femtosecond lasers has revolutionized many areas of science from solid state physics to biology. This new research frontier of ultra-fast VUV and X-ray science drives the development of a novel source for the generation of femtosecond pulses.

In 2012, scientists working on the LCLS overcame the seeding limitation for x-ray wavelengths by self-seeding the laser with its own beam after being filtered through a diamond monochromator. The resulting intensity and monochromaticity of the beam are unprecedented and will allow new experiments to be conducted involving manipulating atoms and imaging molecules. Other labs around the world are incorporating the technique into their equipment.